Assimilation of Multiple Satellite Retrievals with Emissions Adjustment to Improve High Resolution Air Quality Forecast Skill and Predictability

21 oct. 2021 13:05
15m
Oral Presentation 3. Data Assimilation Session 3.

Ponente

Arthur Mizzi (NASA Ames Research Center/Universities Space Research Associates)

Descripción

Poor air quality (AQ) is a most pressing international environmental problem. A soon-to-be-operational network of geostationary AQ satellites (GEMS, TEMPO, and Sentinel 5) that will effectively cover the Northern Hemisphere with hourly AQ observations at ~5 km resolution will revolutionize AQ forecasting/data assimilation. I will present preliminary results from two multi-constituent ensemble AQ forecast/assimilation experiments with WRF-Chem/DART: (i) FRAPPE – a 15 km grid space domain covering the western continental US (CONUS); and (ii) COLORADO – a 4 km grid space domain covering Colorado. These experiments will highlight some of the expected benefits from the geostationary array of AQ satellites.
WRF-Chem/DART incorporates the Weather Research and Forecast (WRF) model with on-line chemistry (WRF-Chem) into the ensemble Kalman filter assimilation system known as the Data Assimilation Research Testbed (DART). We assimilate the ground-based AQS CO, O3, NO2, SO2, PM10, and PM2.5 observations together with MOPITT CO, IASI CO, MODIS AOD, OMI NO2, TROPOMI CO, NO2, and synthetic TEMPO NO2 total/partial column and/or profiles retrievals. We use: (i) the state augmentation method for emissions adjustment, and (ii) state-space localization to enable cross-species adjustments by controlling which observations update which state variables.
I will discuss three basis experiments: (i) CONTROL – assimilates only meteorology; (ii) ALLCHEM – same as CONTROL but also assimilates AQS, MOPITT, IASI, MODIS, OMI, TROPOMI and/or synthetic TEMPO; and (iii) EMISADJ – same as ALLCHEM but also includes emissions adjustment. Our results show that: (i) assimilating chemical observations increases AQ forecast skill; (ii) including emissions adjustment increases forecast skill/predictability time; (iii) including emissions adjustment reduces the magnitude and areal extent of the analysis increments; and (iv) assimilation of high-resolution retrievals from TROPOMI and TEMPO increases the magnitude of the increments. Based on the earlier work of my collaborators, we expect that assimilation of high-resolution retrievals will also increase predictability.

Autor primario

Arthur Mizzi (NASA Ames Research Center/Universities Space Research Associates)

Coautores

Dr Mathew Johnson (NASA Ames Research Cente) Dr Aaron Naeger (University of Alabama at Huntsville) Mr Chia Hua Hsu (University of Colorado at Boulder) Prof. Daven Henze (University of Colorado at Boulder) Dr Rajesh Kumar (National Center for Atmospheric Research (NCAR)) Dr Brian McDonald (National Oceanic and Atmospheric Administration (NOAA)) Dr Jeffrey Anderson (NCAR)

Presentation materials